Theory of resonant tunneling through quantum dots in the presence of electron-phonon interaction

Theory of resonant tunneling through quantum dots in the presence of electron-phonon interaction

Superlattices and Microstructures, THEORY 403 Vol. 10, No. 4, 1991 OF RESONANT PRESENCE TUNNELING THKOllGH OF ELECTRON-PHONON QIIANTUM DOTS 1NT...

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Superlattices

and Microstructures,

THEORY

403

Vol. 10, No. 4, 1991

OF RESONANT PRESENCE

TUNNELING THKOllGH OF ELECTRON-PHONON

QIIANTUM DOTS 1NTERACTIC)N

IN THE

P. Selbmann and 0. Ktin Department of Physics. Humboldt Universltv Invalidenstrasse 110. O- 1040 Berlin. FR( i (Received

Structures

where

the

electrons

15 October

of a two-dimensional

1990)

electron

gas are confined

to discon-

nected regions can be fabricated by the use of appropriate gate geometries. The transpolr between these electrostatically defmed quantum dors takes place by tunneling. lising the tunneling Hamiltonian approach we present a theoretical model of the system including electron-phonon interaction. The relevant coupling constants are determmed from realistic wave functions for the expected confinement potentials. The phonon part of the Hamilton nian is diagonalized using a canonical transformation. Starting from the determination of the transmission matrix for the interacting system we caiculare the current-voltage charac teristics for different temperatures and phonon coupling strengths

1. INTRODUCTION

Resonant tunneling phenomena and their poapplications (fast switches, device tential etc.) have been demonstrated for transistors, structures planar barrier various 111. it has become possible to produce Recently, quasi-one-dimensional (QlD) and quasi-zerodimensional (QOD) electron systems. quantum and dots, by nanolithowires respectively, Transport gra.phg measurements for single quantum dot resonant tunneling structures so far have been reported for two different configurations. Reed et al. 121 use deep etched quantum dots, based on modulation doped GaAs heterostructures, .AIGaAs’InGaAs -multilayer relatively level spacing of with a large about 25 meV. In comparison. electrostatically defined quantum dots in patterned gate structures [3,4] have the advantage of a tunable confinement potential in the plane of the two-dimensional electron gas. But. since is in these devices the dot level spacing typically of t.he order of only some meV their operation is restricted to low temperatures and small voltages. Generally, properties of the tunneling such systems are determlned by their specific takes elertronic structure. The tunneling contacts via place between QlD-states in the localized QOD-levels in the dot: only the is conserved in such a electron total energy process. The obserl,ability of resulting resonance peaks and negative dIPferentia1 conductivitbin the I-V-characteristics - and thus the practical applicability of the devices -

0749-6036/91/080403+04$02.00/0

is mainly controlled by temperature effects the resonant states to and coupling of lattice \,ibrations. In the present paper we use the tunneling Hamiltonian approach (51 to resonant tunneling to develop a sequential theoretical for realistic simple model quantum dot structures which takes these into effects account. Numerical results are presented which correspond to the case of a split gate quantum dot device. In the concluding discussion we give some suggeslions for further work.

2. ELECTRONIC

STATES

An accurate model for any quantum dot structure would require the self-consistent solution of Schroedinger’s equation and Poisson’s equation. Due to the complicated boundar! conditions and the difflcultles of problem in low-dimensional the screening this is an extensive task which is systems, beyond the scope of the present paper inwe use a slmpllfled description which stead, the quanthe electrostatic and decouples tum-mechanical parts of the problem. For the two-dlmenslonal quantization in the z-direction we assume the elec$ric quantum limit: is considered. only the lowest subband, E 0, The electrons of the two-dimensional electron gas (in the x-y plane) are confined by potential self-consistent the superimposed V(x.y). It has been shown by numerical 161 that \‘(x.y) and analytical 171 calculations

0 1991 Academic

Press

Limited

Superlattices

404

can be approximated for not too high carrier so

*2

2

V(x,y)

X

quency

x

x

2

(r=x,y)).

The

eigenfunctions,

E

of

-

2DEG.

n.m=0.1.2

ground

wave

harmonic

is

N

are

easily

found.

(2’)

state

H,(yrr)

function are

F

the

oscillator

of

the

normalized stat,es

subdivided into full Hamiltonlan,

regions is H.

5

0

+ Hra

+ HT

(1)

where

(51

H 0 = HL + Ha + H u is the Hamiltonian the ticles in (wires), and the They are assumed from each other, term. Each contact chemical potential. equals the applied

for non-interacting parcontacts right left and dot region, respectivelyto be completely independent i.e. they commute term by is characterised by its the dif$ereace of which voltage. Er-Er=eU

contains the free phonons PH interaction, electron-phonon which stricted to the dominant coupling lized dot states in our model: H

and

rhe

is

reloca-

to

2 (3)

e a

nnlo’

+ hOy(rn+i)

-rfr’ = S,

Y

(2)

.). The

one-dimensional

where

CURRENT

Schroedinger’s

@0(z)

F,(Y)

= E’ + hw (n+i) x 0

(@0(z)

fre-

wr -characteristic

“In0 for this potential dot we have = F”(x)

H = H

wire

mass,

I nmo(~,y,~)

F,(r)

OF THE TUNNELING

The system is The (see flg.1). written as

dot

*y

2

eigenvalues,

equation For the

“In0

+

2

3. CALCULATION

Vol. IO, No, 4, 1997

(1)

cm*-effectice

E

*2 !JJ (3

least

(at

= *2 mcr 2

and

x

2

by parabolas densities).

and Microstructures,

normalization

y =(m*w poly, and H , is the Hermite r r :h) nomial (r=x,y). In the case of the wire the free motion in the y-dlrection is described by the corresponding plane wave expressions (with the ID wave vector, k) In (2). exp(iky)

(hzk2~2m*), respectively. In the following section we Hamiltonian tunneling method electronic states.

-

(bfr,b

constant,

’ l/2

operayors

operators,

dot

states

c+c

1 i

i.

-

i=n,m.

electron M,,(q)

coupling matrix). This contribution pan be diagonalized exactly by a polaron transe.g. formation (see The remaining 1811. transfer part

and

wlll apply the these using

phonon for

Hr=

c

T

Ir”,rn”’

k,n %“’

a

+

+ T r.,~n.d:ncmn,+ k “Clnn’ c k.n In,“’

h.c

(7)

(a:”(dt,)

-

creation

operator

for

electron

state with wave vector h in subband n in the left (rigth) contact) describes the tunneling between wire and dot states. The transition matrix elements T, for tunneling from region

I to region T

1J

=

!f* 2m

j is ca;iulated

according

/dS

‘4, VY’:)

(‘4: V Y Y J

to

151 (8)

where the integral is taken on a surface in the separating both barrier regions. The application of the transfer matrix method 191, which guarantees continuity of the proyields bability current, with the wave functions given by (2) Flgure I: Idealized energy band model for coupled quantum dot structure under bias direction).

the (Y-

(9)

Superlattices

and Microstructures,

where

-2wax 16k

ray

quires equals

e



40.5

Vol. 10, No. 4, 1991

1

Her; v is r=(2m (Us-E),h the

wave

) in

length.

derivative

region The

with

barrier and dot the plane y=y

electron velocity. decay- constant of

1s the

function

normalization the

tJi$,aclassical

II

prime

(IV). on

respect

to

F

LY is

.

I to region

region

;d& oorl(m.n’I.E’I

III this

6(E+%

J2n

(13)

IIII-”

This condition is used occupation number S(E) for thus the total current

a

WI yry.

The in III

(III and IV) standard The current is calculated by perturbation theory to lowest order with respect to HT 181. For the tunneling current from

I-111

redot

4. RESULTS

to the

determine dot levels

the and

AND DISCUSSION

denotes

wave functions are matched between the regions II and

0

For a stationary system contlnulty that the outgolng current from the the Incoming current

yields

-E’Ilnr(E)-E(E’II

calculated numerically the I-V We have characteristics of quantum dot structures with typical parameters for a split gate device. In figure 2 It is shown how different wlre subbands contribute to the full characteristics. Each channel carries current only as long as the voltage dependent position of the resonance levels in the dot is above the corresponding subband edge. The steep descent of the curves is due to the fact that the tinewidth becomes off-resonant. The Fermi energy In the leads determines the heights and the positions of the peaks. In figure 3 we have plotted the I-V curves for two different temperatures. Any structure in the curves is washed out when the temperature becomes comparable to the dot level spacing,

(10) 4

(n

F -

number) tained spectral

Fermi

distribution,

5

-

dot

occupation

in

All the essential physics are conthe spectral densities, SB. The wire density, dy,a~[(k.n).E], is that of

an ID free particle of energy vector k in subband n. The combined effect of both electron-phonon Interaction on represented tegral [ IO]

a oo,l(m.nl,El=

in

form

J

E

wave 10

type

L I I___& I

I

0

0

in-

‘\

I

c

20

tunneling and looT can be

of a convolution

rmn(E)

with

0

/‘\

-.

iQ 30

,’ --------. 5

A

‘!

10

UlmV-

+

,J,‘mV

-.

r4,,nl(m.nl,E’l (111

dE’ (E-E’)‘+P~(E)

where

I,,,(E)

= n ~\T_j’

is the tunneling.

intrinsic den

6(E-Ern,)

is

level the

broadening dot spectral

(12)

due to density

interactlon electron-phonon intludlng only simplest on the Here we concentrate II II case of a single Einstein model of phonons with energy ho=36 meV for GaAs. It should be mentioned, broadening for

that the phonon induced 1s negligible compared to

a11 temperatures

of interest

level I,,(E)

Figure 2: Resonant tunneling current via three lowest dot levels. Contributions of wire subbands n=O (a). n=l (b). n=2 (cl. the total current cd). Quantum numbers of dot levels are m=l (solid), m=2 (dashed). m=3 (dashed-dotted); (wb=180nm,wa=25nm, Us=22meV, wire:

Er=5meV;

1.5meV.

T=3K)

level

spacing

dot

the the and the and

2.5meV.

406

Superlattices

for different Figure 3: Tunneling current temperatures (a) T=2.5K, (b) T=5K (parameters see fig. 2a, the fourth dot level is included here).

and Microstructures,

Vol. IO, No. 4, 199 7

strength, g=O.O5, the polaron shift is large enough to bring the lowest dot level out of resonance; the corresponding feature at low still seen curve disvoltages, in (a), appears. These few examples show that the proposed model can be used to calculate the I-V characteristics for multi-channel quantum dot resonant tunneling structures with electroncoupling at phonon finite temperatures. It can be combined with a selfconsistent deterthe mination of the relative position of energy levels [21 to simulate real devices Further extensions could be made by lnclusion of level mixing effects [12l due to the real confinement potential profile and coupling to dispersive (acoustic) phonons.

REFERENCES

Ill

i

10

121

: 05

[31

I41 Figure 4: Resonant tunneling current via the two lowest dot levels wlth coupling to LO phonons. Coupling strength: (a) g=O.O25. (b) g=O.O5 (wo=170nm, ws=lOnm. Us=53meV, Er=4meV. level

spacing

dot:

4meV.

wire:

lmeV,

I51

T=6K) 161

The effect of the electronas expected. phonon interaction is demonstrated for two coupling strengths in figure 4. different Although the phonon Induced broadening is still small compared to Pmn(E) we observe the occurence

of

phonon

sidebands

’ in

the

levels.

For

the

higher

181 191

the

transmission. The corresponding current Is about one order of magnitude smaller than the contribution. In addition, the zero phonon curves are shifted by a voltage which equals the polaron shift ghw,, (g-coupling strength) of

171

coupling

1101 1111 1121

Y.0 Cho. F.Capasso. K.Mohammed, and IEEE Journal of Quantum Electronics QE-22,1853,(1986). J.N.Randall. J.H.Luscombe. M.A.Reed, R.J.Matyi. W.R.Frensley, R.J.Aggarwal, T.M.Moore, and A.E.Wetsel. Advances in Solid State Physics 29.267,(1989). B.J.van Wees, H.van Houten. C.W.J.Beenakker, J.W.WillIamson,L.P Kouwenhoven. D.van Marel. and C.T.Foxon. Physical Review Letters 60,848,(1988). H.Ahmed.J.E.Frost, C.G.Smith, M.Pepper, D A.Ritchie. D.G.Hasko, D.C.Peacock, and G.A.C.Jones, Superlattices and Microstructures 6,599,(1989). C.B.Duke, Solid State Physics 10,edited by F.Seitz, D.Turnbull, and H.Ehrenreich, Academic Press, London and New York 1969. SurS.E.Laux. D.J.Frank, and F.Stern, face Science 191,101.(1988). J.H.Davles, Semiconductor Science and Technology 3,995,(1988). G.D.Mahan, “4lany Particle Ph~x~c’s’. flenum Press, New York and London, 1981 E.O.Kane in “Tunneling Phenomena in Soljds”. edited by E.Burstein and 1) Lundquist. Plenum Press, New York. 1969 C.O.Almbladh and P.Minnhagen, Physical Review B 17,929,(1978) C.B.Duke and G.D.Mahan. Physical Keview 139,A1965,(1965). C.W.Bryant. Physical Review B 39. 3145. (1989).